{"doi":"10.1038/s44160-024-00623-4","title":"Forging out-of-equilibrium supramolecular gels","abstract":"The design of supramolecular hydrogels comprising aligned domains is important for the fabrication of biomimetic materials and applications in optoelectronics. One way to access such materials is by the self-assembly of small molecules into long fibres, which can be aligned using an external stimulus. Out-of-equilibrium supramolecular gels can also be designed, where pre-programmed changes of state can be induced by the addition of chemical fuels. Here we exploit these dynamic properties to form materials with aligned domains through a 'forging' approach: an external force is used to rearrange the underlying network from random to aligned fibres as the system undergoes a pre-programmed gel-to-sol-to-gel transition. We show that we can predictably organize the supramolecular fibres, leading to controllable formation of materials with aligned domains through a high degree of temporal control.","journal":"Nature Synthesis","year":2024,"id":423887,"datarank":0.0,"base_score":0.0,"endowment":0.0,"self_citation_contribution":0.0,"citation_network_contribution":0.0,"self_endowment_contribution":0.0,"citer_contribution":0.0,"corpus_percentile":null,"corpus_rank":null,"citation_count":23,"citer_count":0,"citers_with_citation_signal":0,"citers_with_endowment":0,"datacite_reuse_total":0,"is_dataset":false,"is_dataset_confidence":0.9492,"is_data_producer":false,"deposit_databanks":null,"is_oa":true,"file_count":0,"downloads":0,"has_version_chain":false,"published_date":"2024-01-01","fair_score":null,"fair_percentile":null,"algorithm_id":"datarank_citation_only_1hop_v6","ranking_scope":"data_only","authors":[{"id":1219687,"name":"Fin Hallam Stewart","orcid":"0009-0009-8761-2678","position":1,"is_corresponding":false},{"id":1219688,"name":"Santanu Panja","orcid":"0000-0002-5082-5196","position":2,"is_corresponding":false},{"id":1220231,"name":"Asra Zyar","orcid":null,"position":3,"is_corresponding":false},{"id":1219689,"name":"Emma Bowley","orcid":"0009-0008-2771-6857","position":4,"is_corresponding":false},{"id":1219690,"name":"Marko Bek","orcid":"0000-0001-6405-8541","position":5,"is_corresponding":false},{"id":1219691,"name":"Roland Kádár","orcid":"0000-0002-6255-4952","position":6,"is_corresponding":false},{"id":1219692,"name":"Ann E. Terry","orcid":"0000-0003-1105-0372","position":7,"is_corresponding":false},{"id":1220232,"name":"Roberto Appio","orcid":null,"position":8,"is_corresponding":false},{"id":1219693,"name":"Tomás S. Plivelic","orcid":"0000-0003-0193-3251","position":9,"is_corresponding":false},{"id":1220233,"name":"M.C. Maguire","orcid":null,"position":10,"is_corresponding":false},{"id":454917,"name":"Harish Poptani","orcid":"0000-0002-0593-3235","position":11,"is_corresponding":false},{"id":692121,"name":"Marco Marcello","orcid":"0000-0002-2392-8640","position":12,"is_corresponding":false},{"id":513137,"name":"Ravi R. Sonani","orcid":"0000-0002-6212-2869","position":13,"is_corresponding":false},{"id":305492,"name":"Edward H. Egelman","orcid":"0000-0003-4844-5212","position":14,"is_corresponding":false},{"id":1219694,"name":"Dave J. Adams","orcid":"0000-0002-3176-1350","position":15,"is_corresponding":false},{"id":1219686,"name":"Simona Bianco","orcid":"0000-0001-5305-8546","position":0,"is_corresponding":true}],"reference_count":68,"raw_metadata":null,"created_at":"2026-07-19T01:58:01.889748Z","pmid":"39664796","pmcid":null,"fwci":null,"citation_percentile":null,"influential_citations":0,"oa_status":null,"license":null,"views":0,"total_file_size_bytes":0,"version_count":0,"fair_f":null,"fair_a":null,"fair_i":null,"fair_r":null,"fair_zscore":null,"fair_rationale":null,"fair_model":null,"fair_agent_version":null,"fair_fulltext_source":null,"fair_has_llm":null,"fair_computed_at":null,"clinical_trials":[],"software_tools":[],"db_accessions":[],"linked_datasets":[],"topics":[]}